All hairsprays are required to no long have Chloroflourocarbons (CFCs) which contribute to the damage of the ozone layer. You just want to make sure you are buying a hair spray that is safe for you which in turn makes it more eco friendly. You want hairsprays without phthalates, formaldehyde, a high level of petroleum products, and synthetic fragrances.
Try making your own hairspray. You can buy spray bottles at the dollar store or re-use empty ones that you wash out. To make your own hair spray, you need 1 lemon and 2 cups of water. Juice the lemons and then add the lemon pieces and the water to the bowl and set the bowl in a pot of simmering water. Simmer the lemon water mixture until it has been reduced by half. Pour it through a piece of cheesecloth to strain out the lemon pieces. Let the liquid cool, and then transfer it to a clean spray bottle.
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