Just as in any building, small steps such as using biodegradable cleaning supplies, reusing cups rather than disposable and recycling are all important and effective. You could even take it a step further and create a vermicompost which can be easily made and kept inside without worry of a nasty smell for all of your organic food waste.
There are a few sites online that can give a checklist of how to make a daycare green. The site below has a Child Care Checklist that is used by the Oregon Environmental Council for daycare centers.
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