There are lots of documentaries on sustainability, examples of which are The Great Squeeze, A Passion For Sustainability (focuses on Portland, Oregon, named the most sustainable city in the United States), Heart and Soil, and Too Hot Not to Handle.
In addition to those posted by paulataffy, No Impact Man is a documentary about a family trying to erase their carbon footprint 100% for an entire year. For them, this means only self propelled transportation, no electricity, and no toilet paper! Very fun and interesting to watch.
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